Please use this identifier to cite or link to this item: http://hdl.handle.net/10397/81769
PIRA download icon_1.1View/Download Full Text
DC FieldValueLanguage
dc.contributorDepartment of Applied Biology and Chemical Technology-
dc.creatorWang, J-
dc.creatorHan, LL-
dc.creatorHuang, BL-
dc.creatorShao, Q-
dc.creatorXin, HLL-
dc.creatorHuang, XQ-
dc.date.accessioned2020-02-10T12:29:05Z-
dc.date.available2020-02-10T12:29:05Z-
dc.identifier.urihttp://hdl.handle.net/10397/81769-
dc.language.isoenen_US
dc.publisherNature Publishing Groupen_US
dc.rightsOpen Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in thearticle’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.en_US
dc.rights© The Author(s) 2019en_US
dc.rightsThe following publication Wang, J., Han, L., Huang, B. et al. Amorphization activated ruthenium-tellurium nanorods for efficient water splitting. Nat Commun 10, 5692 (2019), 1-11 is available at https://dx.doi.org/10.1038/s41467-019-13519-1en_US
dc.titleAmorphization activated ruthenium-tellurium nanorods for efficient water splittingen_US
dc.typeJournal/Magazine Articleen_US
dc.identifier.spage1-
dc.identifier.epage11-
dc.identifier.volume10-
dc.identifier.doi10.1038/s41467-019-13519-1-
dcterms.abstractPursuing active and durable water splitting electrocatalysts is of vital significance for solving the sluggish kinetics of the oxygen evolution reaction (OER) process in energy supply. Herein, theoretical calculations identify that the local distortion-strain effect in amorphous RuTe2 system abnormally sensitizes the Te-p pi coupling capability and enhances the electron-transfer of Ru-sites, in which the excellent inter-orbital p-d transfers determine strong electronic activities for boosting OER performance. Thus, a robust electrocatalyst based on amorphous RuTe2 porous nanorods (PNRs) is successfully fabricated. In the acidic water splitting, a-RuTe2 PNRs exhibit a superior performance, which only require a cell voltage of 1.52 V to reach a current density of 10 mA cm(-2). Detailed investigations show that the high density of defects combine with oxygen atoms to form RuOxHy species, which are conducive to the OER. This work offers valuable insights for constructing robust electrocatalysts based on theoretical calculations guided by rational design and amorphous materials.-
dcterms.accessRightsopen accessen_US
dcterms.bibliographicCitationNature communications, 12 Dec. 2019, v. 10, 5692, p. 1-11-
dcterms.isPartOfNature communications-
dcterms.issued2019-
dc.identifier.isiWOS:000502254500001-
dc.identifier.scopus2-s2.0-85076352246-
dc.identifier.pmid31831748-
dc.identifier.eissn2041-1723-
dc.identifier.artn5692-
dc.description.validate202002 bcrc-
dc.description.oaVersion of Recorden_US
dc.identifier.FolderNumberOA_Scopus/WOSen_US
dc.description.pubStatusPublisheden_US
Appears in Collections:Journal/Magazine Article
Files in This Item:
File Description SizeFormat 
Wang_Amorphization_Activated_Ruthenium-tellurium.pdf4.2 MBAdobe PDFView/Open
Open Access Information
Status open access
File Version Version of Record
Access
View full-text via PolyU eLinks SFX Query
Show simple item record

Page views

100
Citations as of Jun 26, 2022

Downloads

63
Citations as of Jun 26, 2022

SCOPUSTM   
Citations

109
Citations as of Jun 30, 2022

WEB OF SCIENCETM
Citations

103
Citations as of Jun 30, 2022

Google ScholarTM

Check

Altmetric


Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.