Please use this identifier to cite or link to this item:
http://hdl.handle.net/10397/95734
DC Field | Value | Language |
---|---|---|
dc.contributor | Department of Mechanical Engineering | en_US |
dc.creator | Shi, X | en_US |
dc.creator | Huo, X | en_US |
dc.creator | Esan, OC | en_US |
dc.creator | Dai, Y | en_US |
dc.creator | An, L | en_US |
dc.creator | Zhao, TS | en_US |
dc.date.accessioned | 2022-10-05T03:56:42Z | - |
dc.date.available | 2022-10-05T03:56:42Z | - |
dc.identifier.issn | 1944-8244 | en_US |
dc.identifier.uri | http://hdl.handle.net/10397/95734 | - |
dc.language.iso | en | en_US |
dc.publisher | American Chemical Society | en_US |
dc.rights | © 2022 American Chemical Society | en_US |
dc.rights | This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Applied Materials & Interfaces, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://dx.doi.org/10.1021/acsami.2c03203. | en_US |
dc.subject | E-fuel | en_US |
dc.subject | Fuel cell | en_US |
dc.subject | Stack | en_US |
dc.subject | Water flooding | en_US |
dc.subject | Water management | en_US |
dc.title | Manipulation of electrode composition for effective water management in fuel cells fed with an electrically rechargeable liquid fuel | en_US |
dc.type | Journal/Magazine Article | en_US |
dc.identifier.spage | 18600 | en_US |
dc.identifier.epage | 18606 | en_US |
dc.identifier.volume | 14 | en_US |
dc.identifier.issue | 16 | en_US |
dc.identifier.doi | 10.1021/acsami.2c03203 | en_US |
dcterms.abstract | The liquid fuel cell, with its high energy density and ease of fuel handling, has attracted great attention worldwide. However, its real application is still being greatly hindered by its limited power density. Hence, the recently proposed and demonstrated fuel cell, using an electrically rechargeable liquid fuel (e-fuel), is believed to be a candidate with great potential due to its significant performance advancement. Unlike the conventional alcoholic liquid fuels, the e-fuel possesses excellent reactivity, even on carbon-based materials, which therefore allows the e-fuel cell to achieve superior performance without any noble metal catalysts. However, it is found that, during the cell operation, the water generated at the cathode following the oxygen reduction reaction could lead to a water flooding problem and further limit the cell performance. To address this issue, in this work, by manipulating the cathode composition, a blended binder cathode using both Nafion and polytetrafluoroethylene as binding agents is fabricated and demonstrated its superiority in the fuel cell to achieve an enhanced water management and cell performance. Furthermore, using the developed cathode, a fuel cell stack is designed and fabricated to power a 3D-printed toy car, presenting this system as a promising device feasible for future study and real applications. | en_US |
dcterms.accessRights | open access | en_US |
dcterms.bibliographicCitation | ACS applied materials and interfaces, 27 Apr. 2022, v. 14, no. 16, p. 18600-18606 | en_US |
dcterms.isPartOf | ACS applied materials and interfaces | en_US |
dcterms.issued | 2022-04-27 | - |
dc.identifier.scopus | 2-s2.0-85128998896 | - |
dc.identifier.pmid | 35420776 | - |
dc.identifier.eissn | 1944-8252 | en_US |
dc.description.validate | 202210 bckw | en_US |
dc.description.oa | Accepted Manuscript | en_US |
dc.identifier.FolderNumber | a1728 | - |
dc.identifier.SubFormID | 45844 | - |
dc.description.fundingSource | RGC | en_US |
dc.description.pubStatus | Published | en_US |
Appears in Collections: | Journal/Magazine Article |
Files in This Item:
File | Description | Size | Format | |
---|---|---|---|---|
Shi_Electrode_Composition_Fuel.pdf | Pre-Published version | 3.21 MB | Adobe PDF | View/Open |
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