Please use this identifier to cite or link to this item: http://hdl.handle.net/10397/95367
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dc.contributorDepartment of Applied Biology and Chemical Technologyen_US
dc.creatorYang, Qen_US
dc.creatorMa, Wen_US
dc.creatorWang, Gen_US
dc.creatorBao, Wen_US
dc.creatorDong, Xen_US
dc.creatorLiang, Xen_US
dc.creatorZhu, Len_US
dc.creatorLee, CSen_US
dc.date.accessioned2022-09-19T01:59:56Z-
dc.date.available2022-09-19T01:59:56Z-
dc.identifier.issn1523-7060en_US
dc.identifier.urihttp://hdl.handle.net/10397/95367-
dc.language.isoenen_US
dc.publisherAmerican Chemical Societyen_US
dc.rights© 2017 American Chemical Societyen_US
dc.rightsThis document is the Accepted Manuscript version of a Published Work that appeared in final form in Organic Letters, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acs.orglett.7b02610.en_US
dc.titleTunable cyclization strategy for the synthesis of Zizaene-, allo-Cedrane-, seco-Kaurane-, and seco-Atesane-Type Skeletonsen_US
dc.typeJournal/Magazine Articleen_US
dc.identifier.spage5324en_US
dc.identifier.epage5327en_US
dc.identifier.volume19en_US
dc.identifier.issue19en_US
dc.identifier.doi10.1021/acs.orglett.7b02610en_US
dcterms.abstractA versatile Lewis acid-mediated cyclization strategy has been developed for selectively establishing zizaene-, allo-cedrane-, seco-kaurane-, and secoatesane- type skeletons. The zizaene- and seco-atesane-type skeletons can be obtained in a cascade manner, which involves Diels-Alder reaction of cyclic enones with bissilyloxy dienes and carbocyclization of yne-enolates through Lewis acid dependent 5- or 6-exo-dig modes. This cyclization strategy was also employed for the core synthesis of tashironin.en_US
dcterms.accessRightsopen accessen_US
dcterms.bibliographicCitationOrganic letters, 6 Oct. 2017, v. 19, no. 19, p. 5324-5327en_US
dcterms.isPartOfOrganic lettersen_US
dcterms.issued2017-10-06-
dc.identifier.scopus2-s2.0-85032659601-
dc.identifier.pmid28933167-
dc.identifier.eissn1523-7052en_US
dc.description.oaAccepted Manuscripten_US
dc.identifier.FolderNumberRGC-B2-1533-
dc.description.fundingSourceRGCen_US
dc.description.fundingSourceOthersen_US
dc.description.fundingTextthe NSFC (National Natural Science Foundation of China; Chinese Postdoctoral Science Foundation; the SSTIC (Shenzhen Science and Technology Innovation Committee; Peking University Shenzhen Graduate Schoolen_US
dc.description.pubStatusPublisheden_US
dc.description.oaCategoryGreen (AAM)en_US
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