Please use this identifier to cite or link to this item:
http://hdl.handle.net/10397/109028
DC Field | Value | Language |
---|---|---|
dc.contributor | Department of Electrical and Electronic Engineering | en_US |
dc.contributor | Research Institute for Smart Energy | en_US |
dc.contributor | Photonics Research Institute | en_US |
dc.contributor | Department of Applied Physics | en_US |
dc.creator | Xie, X | en_US |
dc.creator | Ma, R | en_US |
dc.creator | Luo, Y | en_US |
dc.creator | Dela Peña, TA | en_US |
dc.creator | Fong, PWK | en_US |
dc.creator | Luo, D | en_US |
dc.creator | Chandran, HT | en_US |
dc.creator | Jia, T | en_US |
dc.creator | Li, M | en_US |
dc.creator | Wu, J | en_US |
dc.creator | Kyaw, AKK | en_US |
dc.creator | Li, G | en_US |
dc.date.accessioned | 2024-09-13T07:19:57Z | - |
dc.date.available | 2024-09-13T07:19:57Z | - |
dc.identifier.issn | 1614-6832 | en_US |
dc.identifier.uri | http://hdl.handle.net/10397/109028 | - |
dc.language.iso | en | en_US |
dc.publisher | Wiley-VCH Verlag GmbH & Co. KGaA | en_US |
dc.rights | © 2024 The Author(s). Advanced Energy Materials published byWiley-VCH GmbH. This is an open access article under the terms of theCreative Commons Attribution License (http://creativecommons.org/licenses/by/4.0/), which permits use, distributionand reproduction in any medium, provided the original work is properlycited. | en_US |
dc.rights | The following publication X. Xie, R. Ma, Y. Luo, T. A. Dela Peña, P. W.-K. Fong, D. Luo, H. T. Chandran, T. Jia, M. Li, J. Wu, A. K. K. Kyaw, G. Li, Thickness Insensitive Organic Solar Cells with High Figure-of-Merit-X Enabled by Simultaneous D/A Interpenetration and Stratification. Adv. Energy Mater. 2024, 2401355 is available at https://doi.org/10.1002/aenm.202401355. | en_US |
dc.subject | Nonfused ring acceptor | en_US |
dc.subject | Organic solar cells | en_US |
dc.subject | Power conversion efficiency | en_US |
dc.subject | Sequential deposition | en_US |
dc.subject | Thick film | en_US |
dc.title | Thickness insensitive organic solar cells with high figure-of-merit-X enabled by simultaneous D/A interpenetration and stratification | en_US |
dc.type | Journal/Magazine Article | en_US |
dc.identifier.doi | 10.1002/aenm.202401355 | en_US |
dcterms.abstract | Low cost and printing friendly fabrication of organic solar cells (OSCs) require thick-film devices with simply structured photoactive molecules. Thus, achieving high power conversion efficiency (PCE) for non-fused ring acceptor-based devices with high thickness is of great significance. Herein, by transforming traditional blend casting method to emerging sequential deposition (SD) method, D18:A4T-16 active blend exhibits large efficiency improvement from 8.02% to 14.75% in 300 nm thick devices. Systematic morphological and photophysical characterizations showcase the effectiveness of SD processing in achieving sufficient donor/acceptor interpenetration and vertical stratification, which eliminates the dilemma of charge generation/transport in blend casting films. Meanwhile, D18 bottom layer is proven helpful in realizing fast evaporation of postdeposited poor solvent, resulting in naturally thickened active layer with well-regulated crystallization. Furthermore, a new index to emphasize thick-film devices based on nonfused ring acceptors, called figure-of-merit-X (FoM-X), has been defined. The SD processed D18:A4T-16 devices herein, with 300 nm, 500 nm, and 800 nm thicknesses possess leading FoM-X values. | en_US |
dcterms.accessRights | open access | en_US |
dcterms.bibliographicCitation | Advanced energy materials, First published: 14 June 2024, Early View, 2401355, https://doi.org/10.1002/aenm.202401355 | en_US |
dcterms.isPartOf | Advanced energy materials | en_US |
dcterms.issued | 2024 | - |
dc.identifier.scopus | 2-s2.0-85195858845 | - |
dc.identifier.eissn | 1614-6840 | en_US |
dc.identifier.artn | 2401355 | en_US |
dc.description.validate | 202409 bcch | en_US |
dc.description.oa | Version of Record | en_US |
dc.identifier.FolderNumber | OA_TA | - |
dc.description.fundingSource | RGC | en_US |
dc.description.fundingSource | Others | en_US |
dc.description.fundingText | Shenzhen Science and Technology Innovation Commission; Hong Kong Polytechnic University: Sir Sze-yuen Chung Endowed Professorship Fund; RISE; PRI; Guangdong-Hong Kong-Macao Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and Devices; PolyU Distinguished Postdoctoral Fellowship; Natural Science Foundation of Guangdong Province; National Natural Science Foundation of China; Guangdong government; Guangzhou government; Guangzhou Municipal Science and Technology Project; HKUST Materials Characterization and Preparation Facility Guangzhou | en_US |
dc.description.pubStatus | Early release | en_US |
dc.description.TA | Wiley (2024) | en_US |
dc.description.oaCategory | TA | en_US |
Appears in Collections: | Journal/Magazine Article |
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Xie_Thickness_Insensitive_Organic.pdf | 2.83 MB | Adobe PDF | View/Open |
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