Please use this identifier to cite or link to this item:
http://hdl.handle.net/10397/105426
DC Field | Value | Language |
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dc.contributor | Department of Applied Physics | - |
dc.contributor | Research Institute for Smart Energy | - |
dc.creator | Chen, S | en_US |
dc.creator | Ying, Y | en_US |
dc.creator | Ma, L | en_US |
dc.creator | Zhu, D | en_US |
dc.creator | Huang, H | en_US |
dc.creator | Song, L | en_US |
dc.creator | Zhi, C | en_US |
dc.date.accessioned | 2024-04-12T06:52:22Z | - |
dc.date.available | 2024-04-12T06:52:22Z | - |
dc.identifier.uri | http://hdl.handle.net/10397/105426 | - |
dc.language.iso | en | en_US |
dc.publisher | Nature Publishing Group | en_US |
dc.rights | © The Author(s) 2023 | en_US |
dc.rights | Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. | en_US |
dc.rights | The following publication Chen, S., Ying, Y., Ma, L. et al. An asymmetric electrolyte to simultaneously meet contradictory requirements of anode and cathode. Nat Commun 14, 2925 (2023) is available at https://doi.org/10.1038/s41467-023-38492-8. | en_US |
dc.title | An asymmetric electrolyte to simultaneously meet contradictory requirements of anode and cathode | en_US |
dc.type | Journal/Magazine Article | en_US |
dc.identifier.volume | 14 | en_US |
dc.identifier.doi | 10.1038/s41467-023-38492-8 | en_US |
dcterms.abstract | One of the major obstacles hindering the application of zinc metal batteries is the contradictory demands from the Zn metal anode and cathodes. At the anode side, water induces serious corrosion and dendrite growth, remarkably suppressing the reversibility of Zn plating/stripping. At the cathode side, water is essential because many cathode materials require both H+ and Zn2+ insertion/extraction to achieve a high capacity and long lifespan. Herein, an asymmetric design of inorganic solid-state electrolyte combined with hydrogel electrolyte is presented to simultaneously meet the as-mentioned contrary requirements. The inorganic solid-state electrolyte is toward the Zn anode to realize a dendrite-free and corrosion-free highly reversible Zn plating/stripping, and the hydrogel electrolyte enables consequent H+ and Zn2+ insertion/extraction at the cathode side for high performance. Therefore, there is no hydrogen and dendrite growth detected in cells with a super high-areal-capacity up to 10 mAh·cm-2 (Zn//Zn), ~5.5 mAh·cm-2 (Zn//MnO2) and ~7.2 mAh·cm-2 (Zn//V2O5). These Zn//MnO2 and Zn//V2O5 batteries show remarkable cycling stability over 1000 cycles with 92.4% and over 400 cycles with 90.5% initial capacity retained, respectively. | - |
dcterms.accessRights | open access | en_US |
dcterms.bibliographicCitation | Nature communications, 2023, v. 14, 2925 | en_US |
dcterms.isPartOf | Nature communications | en_US |
dcterms.issued | 2023 | - |
dc.identifier.scopus | 2-s2.0-85159822205 | - |
dc.identifier.pmid | 37217467 | - |
dc.identifier.eissn | 2041-1723 | en_US |
dc.identifier.artn | 2925 | en_US |
dc.description.validate | 202403 bcvc | - |
dc.description.oa | Version of Record | en_US |
dc.identifier.FolderNumber | OA_Scopus/WOS | - |
dc.description.fundingSource | RGC | en_US |
dc.description.pubStatus | Published | en_US |
dc.description.oaCategory | CC | en_US |
Appears in Collections: | Journal/Magazine Article |
Files in This Item:
File | Description | Size | Format | |
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s41467-023-38492-8.pdf | 3.18 MB | Adobe PDF | View/Open |
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