Please use this identifier to cite or link to this item: http://hdl.handle.net/10397/27375
Title: Enhanced surface-and-interface coupling in Pd-nanoparticle-coated LaAlO3/SrTiO3 heterostructures : strong gas- and photo-induced conductance modulation
Authors: Kim, H
Chan, NY
Dai, JY 
Kim, DW
Issue Date: 2014
Source: Scientific reports, 23 2014, v. 5, no. , p. 1-6
Abstract: Pd nanoparticle (NP) coated LaAlO3/SrTiO3 (LAO/STO) heterointerface exhibits more notable conductance (G) change while varying the ambient gas (N2, H2/N2, and O2) and illuminating with UV light (wavelength: 365 nm) than a sample without the NPs. Simultaneous Kelvin probe force microscopy and transport measurements reveal close relationships between the surface work function (W) and G of the samples. Quantitative analyses suggest that a surface adsorption/desorption-mediated reaction and redox, resulting in a band-alignment modification and charge-transfer, could explain the gas- and photo-induced conductance modulation at the LAO/STO interface. Such surface-and-interface coupling enhanced by catalytic Pd NPs is a unique feature, quite distinct from conventional semiconductor hetero-junctions, which enables the significant conductance tunability at ultrathin oxide heterointerfaces by external stimuli.
Publisher: Nature Publishing Group
Journal: Scientific reports 
EISSN: 2045-2322
DOI: 10.1038/srep08531
Rights: This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder in order to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
The following publication Kim, H., Chan, N., Dai, J. et al. Enhanced Surface-and-Interface Coupling in Pd-Nanoparticle-coated LaAlO3/SrTiO3 Heterostructures: Strong Gas- and Photo-Induced Conductance Modulation. Sci Rep 5, 8531 (2015) is available at https://dx.doi.org/10.1038/srep08531
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