Please use this identifier to cite or link to this item: http://hdl.handle.net/10397/81523
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dc.contributor.authorXia, Men_US
dc.contributor.authorWang, Wen_US
dc.contributor.authorWang, Zen_US
dc.contributor.authorGao, Jen_US
dc.contributor.authorLi, Hen_US
dc.contributor.authorLiang, Yen_US
dc.contributor.authorYu, Cen_US
dc.contributor.authorZhang, Yen_US
dc.contributor.authorWang, Pen_US
dc.contributor.authorZhang, Yen_US
dc.contributor.authorBi, Fen_US
dc.contributor.authorCheng, Xen_US
dc.contributor.authorWang, Ten_US
dc.date.accessioned2019-10-28T05:45:55Z-
dc.date.available2019-10-28T05:45:55Z-
dc.date.issued2019-
dc.identifier.citationAtmosphere, 2019, v. 10, no. 4, 204en_US
dc.identifier.issn2073-4433-
dc.identifier.urihttp://hdl.handle.net/10397/81523-
dc.description.abstractThe uptake of dinitrogen pentoxide (N2O5) on aerosols affects the nocturnal removal of NOx and particulate nitrate formation in the atmosphere. This study investigates N2O5 uptake processes using field observations from an urban site in Beijing during April-May 2017, a period characterized by dry weather conditions. For the first time, a very large N2O5 uptake rate (k(N2O5) up to ~0.01 s-1) was observed during a sand storm event, and the uptake coefficient ( (N2O5)) was estimated to be 0.044. The γ(N2O5) in urban air masses was also determined and exhibited moderate correlation (r = 0.68) with aerosol volume to surface ratio (Va/Sa), but little relation to aerosol water, nitrate, and chloride, a finding that contrasts with previous results. Several commonly used parameterizations of γ(N2O5) underestimated the field-derived γ(N2O5). A new parameterization is suggested for dry conditions, which considers the effect of Va/Sa, temperature, and relative humidity.en_US
dc.description.sponsorshipDepartment of Civil and Environmental Engineeringen_US
dc.language.isoenen_US
dc.publisherMolecular Diversity Preservation International (MDPI)en_US
dc.relation.ispartofAtmosphereen_US
dc.rights© 2019 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).en_US
dc.rightsThe following publication Xia M, Wang W, Wang Z, Gao J, Li H, Liang Y, Yu C, Zhang Y, Wang P, Zhang Y, Bi F, Cheng X, Wang T. Heterogeneous Uptake of N2O5 in Sand Dust and Urban Aerosols Observed during the Dry Season in Beijing. Atmosphere. 2019; 10(4):204, is available at https://doi.org/10.3390/atmos10040204en_US
dc.subjectAerosol compositionsen_US
dc.subjectN2O5 uptakeen_US
dc.subjectParticle sizeen_US
dc.subjectSand dusten_US
dc.titleHeterogeneous uptake of N2O5 in sand dust and urban aerosols observed during the dry season in Beijingen_US
dc.typeJournal/Magazine Articleen_US
dc.identifier.volume10-
dc.identifier.issue4-
dc.identifier.doi10.3390/ATMOS10040204-
dc.identifier.scopus2-s2.0-85069818665-
dc.identifier.artn204-
dc.description.validate201910 bcma-
dc.description.oapublished_final-
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